环境与化学工程

三峡库区干流及库湾支流(朱衣河)夏季CO2 分压及扩散通量

展开
  • 1. 上海大学环境与化学工程学院, 上海200444;
    2. 华东师范大学河口海岸学国家重点实验室, 上海200062
汪福顺(1976—), 男, 教授, 博士, 研究方向为地球化学. E-mail: fswang@shu.edu.cn

收稿日期: 2015-05-21

  网络出版日期: 2016-08-30

基金资助

国家水体污染控制与治理科技重大专项(2012ZX07104-001); 国家自然科学基金资助项目(41273128, 41473082)

Partial pressure and diffusion flux of dissolved carbon dioxide in mainstream and tributary (Zhuyi River) of the Three Gorges Reservoir in summer

Expand
  • 1. School of Environmental and Chemical Engineering, Shanghai University, Shanghai 200444, China;
    2. State Key Laboratory of Estuarine and Coastal Research, East China Normal University, Shanghai 200062, China

Received date: 2015-05-21

  Online published: 2016-08-30

摘要

以三峡库区中长江干流及其支流朱衣河作为主要研究对象, 于2013 年5—7 月对该研究区域干支流的CO2 分压进行了研究, 并计算出CO2 的扩散通量. 研究结果表明, 在水体剖面上表层水体CO2 分压最小; 随着水深增加, CO2 分压急剧增大, 到达10 m 后才保持稳定. 干支流表层水体CO2 分压的分布和扩散通量差异显著. 5—7 月, 干流水体表层CO2分压为220.8~268.0 Pa, CO2扩散通量为51.05 mmol·m−2·d−1; 支流水体表层CO2 分压为14.9~190.3 Pa, 3 个月的CO2 扩散通量分别为0.42, −0.12 和20.83 mmol·m−2·d−1. 研究结果表明, 支流释放的CO2 远小于干流.

本文引用格式

魏浩斌1, 吴学谦1, 操满1, 傅家楠1, 贾晓斌1, 邓兵2, 汪福顺1 . 三峡库区干流及库湾支流(朱衣河)夏季CO2 分压及扩散通量[J]. 上海大学学报(自然科学版), 2016 , 22(4) : 497 -504 . DOI: 10.3969/j.issn.1007-2861.2015.01.011

Abstract

The mainstream and tributary of the Three Gorges Reservoir were investigated from May 2013 to July 2013 to understand the distribution of the partial pressure of carbon dioxide. The results show that, along the water column of the tributary (Zhuyi River), the lowest value of the partial pressure of carbon dioxide appears in surface water, and increases rapidly with depth. Below 10 meters in depth, the partial pressure of carbon dioxide becomes stable. There are significant differences of the partial pressure of carbon dioxide in surface water between mainstream and tributaries. During the period of investigation,
the partial pressure of carbon dioxide in the surface water of the mainstream is 220.8~268.0 Pa, with an average CO2 emission fluxes of 51.05 mmol·m−2·d−1. The partial pressure of carbon dioxide in the surface water of tributary (Zhuyi River) is 14.9~190.3 Pa. Emission flux of CO2 in the three months are 0.42, −0.12 and 20.83 mmol·m−2·d−1. The result indicates that the tributary Zhuyi River emits less CO2 than the mainstream.

参考文献

[1] Tremblay A, Varfalvy L, Roehm C, et al. Greenhouse gas emissions-fluxes and processes: hydroelectric reservoirs and natural environments [M]. New York: Springer, 2005.
[2] 李双, 王雨春, 操满, 等. 三峡库区库中干流及支流水体夏季二氧化碳分压及扩散通量[J]. 环境科学, 2014, 35(1): 885-891.
[3] Chamberland A, Levesque S. Hydroelectricity, an option to reduce greenhouse gas emissions from thermal power plants [J]. Energy Conversion and Management, 1996, 37(6/7/8): 885-890.
[4] Victor D G. Global warming: strategies for cutting carbon [J]. Nature, 1998, 395: 837-838.
[5] Xing Y P, Xie P, Yang H, et al. Methane and carbon dioxide fluxes from a shallow hypereutrophic subtropical lake in China [J]. Atmospheric Environment, 2005, 39: 5532-5540.
[6] Dos S M A, Rosa L P, Sikar B, et al. Gross greenhouse gas fluxes from hydro-power reservoir compared to thermo-power plants [J]. Energy Policy, 2006, 34(4): 481-488.
[7] Huttunen J T, Vaisanen T S, Hellsten S K, et al. Fluxes of CH4, CO2 and N2O in hydroelectric reservoirs Lokka and Porttipahta in the northern boreal zone in Finland [J]. Global Biogeochemical Cycles, 2002, 16: 1-17.
[8] Raymond P A, Hartmann J, Lauerwald R, et al. Global carbon dioxide emissions from inland waters [J]. Nature, 2013, 503: 355-359.
[9] 姚臣谌, 张靖, 吴以赢, 等. 三峡坝区干流及香溪河库湾水体秋季二氧化碳分压[J]. 生态学杂志, 2012, 31(1): 152-157.
[10] Demarty M, Bastien J, Tremblay A. Annual follow-up of gross diffusive carbon dioxide and methane emissions from a boreal reservoir and two nearby lakes in Qu´ebec, Canada [J]. Biogeosciences, 2011(8): 41-53.
[11] Kelly V. Influence of reserviors on solute transport: a regionalscale approach [J]. Hydrological Processes, 2001, 15(7): 1227-1249.
[12] Huttunen J, Aim J, Liikanen A, et al. Fluxes of methane, carbon dioxide and nitrous oxide in boreal lakes and potential anthropogenic effects on the aquatic greenhouse gas emissions [J]. Chemisphere, 2003, 52(3): 609-621.

[13] Shen Z, Chen L, Hong Q, et al. Assessment of nitrogen and phosphorus loads and causal factors from different land use and soil types in the Three Gorges Reservoir Area [J]. Science of the Total Environment, 2013, 454: 383-392.
[14] Zheng B H, Xiong C J, Liu D F, et al. The influence of hydrodynamic conditions on algal bloom in the Three Gorges Reservoir tributaries [J]. Applied Mechanics and Materials, 2013, 295: 1981-1990.
[15] Zhang Z, Wan C, Zheng Z, et al. Plant community characteristics and their responses to environmental factors in the water level fluctuation zone of the three gorges reservoir in China [J]. Environmental Science and Pollution Research, 2013, 20(10): 7080-7091.
[16] Yang Z J, Liu D F, Ji D B, et al. An eco-environmental friendly operation: an effective method to mitigate the harmful blooms in the tributary bays of Three Gorges Reservoir [J]. Science China Technological Sciences, 2013, 56(6): 1458-1470.
[17] Wang F S, Cao M, Wang B L, et al. Seasonal variation of CO2 diffusion flux from a large subtropical reservoir in East China [J]. Atmospheric Environment, 2015, 103: 129-137.
[18] Cole J, Nina J, Caraco F. Atmospheric exchange of carbon dioxide in a low-wind oligotrophic lake measured by the addition of SF6 [J]. Limnology and Oceanography, 1998, 43(4): 647-656.
[19] Crusius J, Wanninkhof R. Gas transfer velocities measured at low wind speed over a lake [J]. Limnology and Oceanography, 2003, 48(3): 1010-1017.
[20] Wanninkhof R. Relationship between wind speed and gas exchange over the ocean [J]. Journal of Geophysical Research: Oceans (1978—2012), 2014, 12(C5): 351-362.
[21] 梅航远, 汪福顺, 姚臣谌, 等. 万安水库春季二氧化碳分压的分布规律研究[J]. 环境科学, 2011, 32(1): 58-63.
[22] 张永领, 杨小林, 张东. 小浪底水库影响下的黄河花园口站和小浪底站pCO2 特征及扩散通量[J]. 环境科学, 2015, 36: 40-48.
[23] Zhang G L, Zhang J, Ren J L, et al. Distributions and sea-to-air fluxes of methane and nitrous oxide in the North East China Sea in summer [J]. Marine Chemistry, 2008, 110(35): 42-45.

文章导航

/